No. Crosstabs have only one data row. But you have 2 options:
1. If you have Access XP, look at building a pivot table (it's one of the form options). I'm pretty sure you can have more than one data field in that.
2. Build 2 crosstabs, one with the totals and one with the percentages. If the layout is the same you shoukd be able to use a Union query to combine them, and create a report from the query. In the report you can set up teh layout you're after.
There's another, Excel-based option:
3. Build a pivot table in Excel that points at the table / query in Access. You can lay that out as you want for this example. Either: (a) Data | Get External Data and build the query to return data to an Excel worksheet, then base the pivot table on that, or (b) Go Data | Pivot Table, and in the first screen opt to use an external data source. Go through the steps, and then build the pivot table as normal